CO2地质封存源汇匹配及安全性评价进展

doi:10.13809/j.cnki.cn32-1825/te.2023.03.001

摘要/Abstract

摘要：

CCUS是实现碳中和目标的重要技术手段，目前中国正处于“双碳”目标的落实阶段，在CO₂地质封存的经济界限评价、源汇优化和安全监测方面还缺乏成熟的技术体系。从封存技术经济界限、源汇匹配技术、封存安全性及监测3个方面总结了中国CO₂地质封存技术发展历程。回顾了CCUS技术在捕集、运输、注入封存阶段的经济成本，进一步总结了目前各阶段的技术经济界限及其影响因素。此外，通过总结国内外CCUS源汇匹配技术发展现状，明确了中国源汇特征及其分布，提出了进一步开展源汇匹配优化技术的发展方向。最后，通过总结CO₂地质封存安全风险评价及封存监测技术，明确了经济高效、有效、定量的监测方法是未来的研究重点。

关键词: CO₂地质封存, 封存技术经济界限, 源汇匹配, 安全风险评价技术, CO₂泄漏监测技术

Abstract:

CCUS is an important technical means to achieve the carbon neutrality goal. At present, China is in the implementation stage of the “dual carbon” goal, and there is still a lack of mature technical system in the economic boundary assessment, source-sink optimization and safety monitoring of geological sequestration of CO₂. This paper summarizes the development process of China's CO₂ geological sequestration technique from three aspects, economic boundaries of sequestration technology, source-sink matching technology, and sequestration safety and monitoring, reviews the economic costs of CCUS technology in the capture, transportation, injection and burial period, and further summarizes the current technical and economic boundaries and influencing factors of each period. In addition, by summarizing the current development status of CCUS source-sink matching technology at home and abroad, the source-sink characteristics and distribution of China have been clarified, and further development directions for source sink matching optimization technology have been proposed. Finally, by summarizing the safety risk assessment and burial monitoring techniques for geological sequestration of CO₂, it is clear that economically efficient, effective, and quantitative monitoring methods are the focus of future research.

Key words: geological sequestration of CO₂, sequestration technique and economic boundaries, source-sink matching, safety risk assessment technology, CO₂ leakage monitoring technology

中图分类号:

TE122

李士伦,汤勇,段胜才,秦佳正,陈一诺,刘雅昕,郑鹏,赵国庆. CO₂地质封存源汇匹配及安全性评价进展[J]. 油气藏评价与开发, 2023, 13(3): 269-297.

LI Shilun,TANG Yong,DUAN Shengcai,QIN Jiazheng,CHEN Yinuo,LIU Yaxin,ZHENG Peng,ZHAO Guoqing. Progress in source-sink matching and safety evaluation of CO₂ geological sequestration[J]. Petroleum Reservoir Evaluation and Development, 2023, 13(3): 269-297.

图/表 7

图1

图2

图3

图4

表1

表2

表3

不同封堵CO2泄漏监测方法的对比[36]"

监测方法	被测对象	测量类型	测量位置	定位功能	检测精度	区分CO₂来源	泄漏量获得	测量周期
IRGA（红外气体分析仪检测技术）	CO₂体积分数	点测量	地表以上	可确定单点位置	正负 0.2 mL/m3	不能	间接得到	定期或连续
LOIR（长程开放路径红外探测和调制激光检测技术）	CO₂沿程平均体积分数	线测量（几十米至几千米）	地表以上	可根据单个装置位置定位	小于 1 mL/m3	不能	间接得到	定期或连续
AC（集聚气室检测方法）	CO₂小空间平均通量密度	小空间测量/cm²	地表及地表浅层	可根据单个气室位置定位	满量程的正负10 %以内	不能	直接得到	定期或连续
EC（涡量相关监测方法）	CO₂大空间平均通量密度	大空间监测（几平方米到几千平方米）	地表以上	可根据大气条件估算定位	正负 5 %~30 %	不能	直接得到	定期或连续
测井微震法	地下流体流动状态	地质层大范围扫描（几平方米到几百平方米）	地表以下	可根据波动图像判断定位		能	不能得到	定期
无线传感器网络	依赖传感器节点功能	超大范围（几千平方米）	地表以上	精确定位	依赖节点设计	依赖算法	直接得到	连续
LJDAR （激光雷达检测技术）	CO₂大空间平均体积分数	大空间距离（几米到几千米）	地表以上	可根据仪器位置定位	小于 1 mL/m3	不能	间接得到	定期或连续
超光谱成像	地面植被生长状况	大范围（整个大陆面积）	地表以上	可根据成像判断	误差小于20 %	能	不能得到	定期
示踪剂法	示踪剂含量	点测量	地表以上	可根据取样位置定位	依赖示踪剂检测精度	能	间接得到	定期
碳同位素检测	碳同位素值 $（ δ 13 C 、 δ 14 C$ ）	点测量	地表以上或地表浅层	可根据取样位置定位	最大精度可达0.06 %	$δ 13 C$ 能， $δ 14$ C不能	间接得到	定期

表3

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评价对象	指标	指标内涵
盆地	构造特征	构造必须稳定，地震活动少，如前陆盆地，内克拉通盆地等
	水动力条件	水动力系统应具有埋藏深、区域具有一定规模的特点，同时受控于地形、地貌起伏特征
	地热特征	冷盆比热盆更利于CO₂以高密度埋存，增加埋存量
	勘探程度	盆地勘探程度高，具有开发井等详细资料，可为CO₂泄漏监控提供可靠资料
地质体	构造条件	断层、裂缝不发育，斜坡带是有利区带
	盖层条件	为保证长期封存CO₂，盖层厚度、完整性条件非常重要
	规模条件	需具有区域规模
	埋深条件	埋深需要满足CO₂在地下处于临界或超临界状态，同时保证淡水资源的安全
	孔渗条件	需具备高孔隙度、高渗透率特征，以保证CO₂的注入和埋存
	流体性质	溶解埋存、矿化反应是CO₂地下埋存的重要形式，需考虑地层水的矿化度条件
	骨架矿物	储集层条件下CO₂与骨架矿物发生化学反应，形成新的稳定矿物，是CO₂安全埋存的重要形式，埋存量受骨架矿物成分控制

阶段	特点	泄漏路径	控制因素	地质安全界限
阶段	特点	泄漏路径	控制因素	距离断层一个井距以内	距离断层一个井距以外
CO₂驱油阶段	CO₂沿相对高渗透带优先流入采油井井底	开启断层、破裂盖层	断层的重开启压力、盖层的破裂压力	p_gi<p_fr， p_gi<p_cf	p_gi<p_cf
CO₂注入阶段	CO₂通过注入井注入储层	开启断层、破裂盖层、断层岩、盖层	断层的重开启压力、盖层的破裂压力、断层岩纵向封堵压力、盖层封堵压力	p_gi<min（p_fr，p_cf）， p<min（p_fvs，p_cf）	p_gi<min（p_cf，p_cs）
CO₂封存阶段	CO₂充满油藏储层	开启断层、破裂盖层、断层岩、盖层、溢出点	断层的重开启压力、盖层的破裂压力、断层岩纵向封堵压力、盖层封堵压力、油藏最大容量	p<min（p_fr，p_cs）， p<min（p_fvs，p_cs）， Q_s<Q_p

CO₂地质封存源汇匹配及安全性评价进展

Progress in source-sink matching and safety evaluation of CO₂ geological sequestration

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